A modified accumulator method for measuring surface radon flux from a uranium tailings pile

"A modified accumulator method was devised to measure surface radon flux from porous media. It consists of a collector hood type of accumulator with a homogenizer pump and a pressure balancer. The latter was used to compensate any pressure changes produced during sample withdrawal and hence eliminate additional radon transport from the media. Errors resulting from radon back diffusion due to decreasing concentration gradient with time across the interface were also eliminated by measuring radon concentrations in the accumulator for two different periods of time and calculating the true radon flux, J(o), from the solution of a time-dependent radon transport equation in the absence of any pressure and temperature gradients.Core samples from the observation site were also withdrawn for laboratory determination of porosity, moisture content, bulk and grain densities, Ra-226 source concentration and the fraction of Rn-222 produced in the void volume. The data were used to calculate the radon diffusion coefficient for the media.Using the present method, the true value of surface radon flux for an abandoned uranium tailings pile was obtained as J(o) = 2020.2 mBq/m2/sec (54.6 pCi/m2/sec) compared to the value J = 1406.0 mBq/m2/sec (38.0 pCi/m2/sec) obtained by the conventional method. The bulk diffusion coefficient of radon for the media was obtained as 1.2 x 10-7 m2/sec.IntroductionRadon-222 (hereafter called radon) released from uranium mill tailings is a continuous source of environment radioactivity in terms of its transport as an airborne gas and its decay products. The particulate daughter products readily attach to aerosols or dust particles and can further be transported by various other environmental pathways. Typical radon release rates from existing tailings piles vary between 740 and 14,800 mBq/m2/sec (20-400 pCilm2/sec), depending on the nature of the tailings material, moisture content, etc. The United States Nuclear Regulatory Commission (NRC) is proposing radon release rates of 74 mBq/m2/sec (2 pCi/m2/sec) above that of background."